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Research

Materials and Cell Architectures for Safe, Sustainable and High-Performance Energy Storage

Research focused on understanding and engineering the relationships among material structure, surface chemistry, electrochemical interfaces, ion transport and cell-level performance.

Theme 01

Lithium-Sulfur Batteries

Cathode architecture, polysulfide regulation and cell design for sulfur-based lithium cells.

Scientific challenges

  • Poor electrical conductivity of sulfur
  • Polysulfide dissolution
  • Shuttle effect
  • Slow conversion kinetics
  • Electrode-volume changes
  • Capacity degradation
  • Limited practical sulfur loading

Scientific Problem

Sulfur is electronically insulating, its intermediates dissolve into the electrolyte, and conversion kinetics are slow. Together these produce shuttle losses, electrode-volume changes and capacity decay that worsen as practical sulfur loading increases.

Current Research Foundation

Doctoral work at IIT Roorkee produced hierarchical porous carbon hosts, nano-TiO₂-grafted carbon interlayers and MoS₂-functionalised separators, each evaluated in coin cells with post-mortem structural and chemical analysis.

Proposed Research Direction

Extend adsorption-plus-catalysis designs to higher sulfur loading and reduced electrolyte-to-sulfur ratios, and correlate interfacial chemistry with cell-level behaviour rather than coin-cell capacity alone.

Methods and Tools

  • Hierarchical porous carbon hosts
  • Functional interlayers
  • Polar metal oxides
  • Transition-metal sulfides
  • Separator modification
  • Chemical anchoring
  • Catalytic polysulfide conversion
  • Cell-architecture optimisation

Expected Scientific Contribution

A clearer link between host porosity, interfacial catalysis and the durability of sulfur cathodes under practical operating constraints.

Theme 02

Sodium-Sulfur and Sodium-Ion Batteries

Earth-abundant sodium chemistries, cathode materials and interfaces for lower-cost storage.

Scientific Problem

Sodium chemistries offer resource advantages, but larger ionic radius, structural instability during cycling and less stable interfaces limit rate capability and cycle life.

Current Research Foundation

Completed work includes polysulfide-regulation studies extended to Na-S systems within submitted manuscripts, and contribution to cathode-material and solid-state electrolyte-component development for sodium-ion systems during the Project Scientist role at IIT Kanpur (August–November 2025).

Proposed Research Direction

Planned work targets sodium-ion cathode compositions with improved structural reversibility, and systematic study of sodium-ion transport across engineered electrode-electrolyte interfaces. This direction is proposed rather than completed.

Methods and Tools

  • Cathode materials
  • Sodium-ion transport analysis
  • Structural stability studies
  • Electrochemical interfaces
  • Solid-state electrolyte components
  • Rate capability
  • Long-term cycling

Expected Scientific Contribution

Transfer of sulfur-cathode design principles into sodium chemistries, with an explicit separation between demonstrated results and proposed work.

Theme 03

Porous and Biomass-Derived Carbon

Conductive, ion-accessible carbon frameworks obtained from sustainable precursors.

Scientific Problem

Carbon hosts must simultaneously provide electronic conduction, sulfur confinement and open ion pathways. Pore architectures optimised for one function frequently compromise another.

Current Research Foundation

Orange-peel-derived hierarchical porous carbon was synthesised, characterised by BET, XRD, Raman and electron microscopy, and evaluated as a sulfur host in Li-S cells.

Proposed Research Direction

Heteroatom doping and controlled pore hierarchies are being pursued to combine chemical affinity for polysulfides with unobstructed ion access.

Methods and Tools

  • Hierarchical porous structures
  • Heteroatom-doped carbons
  • Biowaste-derived carbon
  • Sulfur encapsulation
  • Ion-accessible pore networks
  • Conductive frameworks
  • Sustainable precursor utilisation

Expected Scientific Contribution

Design rules relating precursor chemistry and activation conditions to electrochemically useful pore architectures.

Theme 04

Functional Separators and Interlayers

Thin functional layers that adsorb, convert and regulate soluble intermediates.

Relevant materials

  • Nano-TiO₂-grafted carbon sheets
  • rGO/MgO composite coatings
  • 2D-MoS₂ nanoflakes
  • Polar catalytic compounds
  • Carbon-based interlayers

Scientific Problem

A conventional separator is electrochemically passive. It permits intermediate migration and offers no route to accelerate the redox conversion of trapped species.

Current Research Foundation

Nano-TiO₂-grafted carbon sheets, rGO/MgO composite coatings and 2D-MoS₂ nanoflakes have been prepared and evaluated as interlayers or separator coatings, with post-mortem analysis of the recovered components.

Proposed Research Direction

Combining adsorptive and catalytic functions within a single low-mass coating, so that regulation is achieved without penalising cell energy density.

Methods and Tools

  • Polysulfide adsorption
  • Shuttle-effect suppression
  • Catalytic conversion
  • Ion transport
  • Redox regulation
  • Interface stabilisation

Expected Scientific Contribution

Quantitative understanding of how coating composition and thickness trade against transport resistance and practical cell metrics.

Theme 05

Solid-State and Quasi-Solid-State Systems

An emerging direction, building on solid-state component work rather than an established programme.

Scientific Problem

Solid electrolytes promise improved safety, but interfacial resistance, chemical incompatibility, dendrite penetration and mechanical integrity remain unresolved at the cell level.

Current Research Foundation

Initial exposure comes from solid-state electrolyte-component development for sodium-ion systems during the Project Scientist role at IIT Kanpur. This is early-stage experience, not an independent research programme.

Proposed Research Direction

Study of electrode-electrolyte compatibility and interfacial resistance in quasi-solid-state configurations, approached incrementally alongside established liquid-electrolyte work.

Methods and Tools

  • Sulfide solid electrolytes
  • Oxide solid electrolytes
  • Electrode-electrolyte compatibility
  • Interfacial resistance analysis
  • Dendrite mitigation
  • Chemical stability
  • Mechanical integrity

Expected Scientific Contribution

Interface-level insight that connects solid-electrolyte chemistry with measurable cell impedance and stability.

Theme 06

Battery Sustainability and Circularity

A long-term pillar linking material sourcing, synthesis and end-of-life recovery.

Scientific Problem

Energy-storage research often optimises performance in isolation from precursor availability, synthesis burden and the recovery of materials from spent cells.

Current Research Foundation

Biowaste-derived carbon work established that low-value agricultural residue can yield functional battery materials through comparatively simple processing.

Proposed Research Direction

Extending sustainable sourcing to earth-abundant electrode compounds, and developing recovery routes that return active materials to useful electrochemical service.

Methods and Tools

  • Biowaste-derived functional materials
  • Earth-abundant electrode compounds
  • Environmentally responsible synthesis
  • Battery-material recovery
  • Recycling of spent cells
  • Reuse of recovered active materials
  • Circular battery-material pathways

Expected Scientific Contribution

Evidence on whether recovered and biowaste-derived materials can meet the electrochemical requirements of practical cells.

Method

Research workflow

A consistent experimental sequence applied across themes, from material choice to mechanism and optimisation.

  1. 01Material Selection
  2. 02Synthesis and Processing
  3. 03Structural and Surface Characterisation
  4. 04Electrode and Cell Fabrication
  5. 05Electrochemical Evaluation
  6. 06Post-Mortem Analysis
  7. 07Mechanism Understanding
  8. 08Performance Optimisation

Research Vision

From Functional Materials to Sustainable Cell-Level Energy Storage

A staged programme that begins with materials already demonstrated in doctoral work and widens, over time, towards interface-engineered full cells and circular battery materials.

  1. 01

    Immediate Research Programme

    First 1–3 years

    • Functional sulfur hosts
    • Advanced separators and interlayers
    • Sodium-ion cathode materials
    • Electrochemical mechanism studies
    • High-loading electrode evaluation
    • Reduced-electrolyte cell configurations
  2. 02

    Medium-Term Programme

    Approximately 3–5 years

    • Solid-state and quasi-solid-state systems
    • Interface-engineered full cells
    • Integrated materials and cell-design strategies
    • Collaborative characterisation and modelling
    • Scalable synthesis approaches
  3. 03

    Long-Term Programme

    Beyond five years

    • Sustainable battery-material systems
    • Battery recycling and resource recovery
    • Interdisciplinary research group development
    • Academic and industrial partnerships
    • Translation from materials discovery to cell validation